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              <p>On Pluto, the largest object in the Kuiper Belt, the dark surface of Cthulhu seems to indicate thepresence of photochemical aerosols, stemming from the interaction between solar ultravioletradiation and atmospheric methane, nitrogen, carbon monoxide, and further sedimentation [1-4].Tholins have been tested and identified as analogues of the said surface. The flyby of the NewHorizons Pluto probe enabled reflectance spectra acquisitions of the Cthulhu region. Dissimilaritieswere found with the reflectance of Pluto tholins, which might be due to Galactic Cosmic Rays (GCR)irradiation of Pluto’s surface [5]. To test this hypothesis, Pluto tholins were synthesized and swiftheavy ion irradiation was performed on the analogues to simulate the impact of cosmic rays on thesurface of Cthulhu region. Moreover, GCR-analogues irradiation of the said tholins triggers adesorption of organic volatile compounds whose study could provide crucial information on both thestructure of tholins and the chemical mechanisms involved. The volatile desorption was followed bymass spectrometry.</p>
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